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JOURNAL OF SYNTHETIC CRYSTALS ›› 2023, Vol. 52 ›› Issue (6): 960-981.

Special Issue: 半导体薄膜与外延技术

• Optoelectronic Thin Films • Previous Articles     Next Articles

Basic Materials and Devices of the Deterministic Solid-State Quantum Light Sources

ZHAO Junyi1,2, LIU Runze1,2, LOU Yiyang1,2, HUO Yongheng1,2,3   

  1. 1. Hefei National Research Center for Physical Sciences at the Microscale and School of Physical Sciences, University of Science and Technology of China, Hefei 230026, China;
    2. Shanghai Research Center for Quantum Science and CAS Center for Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China, Shanghai 201315, China;
    3. Hefei National Laboratory, University of Science and Technology of China, Hefei 230088, China
  • Received:2023-04-09 Online:2023-06-15 Published:2023-06-30

Abstract: Quantum light sources are fundamental modules for quantum communication and optical quantum computation. The quality of quantum light sources directly determines the implementation of quantum key distribution and optical quantum computation. For example, the indivisibility of photons ensures the unconditional security of quantum communication, and the indistinguishability of photons ensures the complexity of computing schemes. Among various solid-state candidate systems, single and entangled photon sources based on solid-state semiconductor quantum dots (QDs) have shown great potential compared to their competitors. Molecular beam epitaxy (MBE) is currently the most suitable technique for growing solid-state semiconductor QDs, with advantages of ultra-high vacuum, ultra-pure materials, in-situ monitoring, and highly controllable growth parameters. To achieve quantum light sources with high efficiency, high single-photon purity, high indistinguishability, and high entanglement fidelity simultaneously, the material growth, external field tuning, surface passivation, and optical measurement techniques of QDs need to be systematically optimized and improved. This article reviews the research progress of basic materials and devices of solid-state QDs systems based on MBE growth. Subsequently, this article discusses the mechanisms of the growth of two types of QDs, the influences of various growth parameters on the quality of QDs, including background vacuum, purity of source materials, substrate temperature, growth rate, beam equivalent pressure (BEP) ratio, etc. After that, this article introduces the technical details and experimental progress of optimizing QDs device performance from the perspectives of external field tuning, surface passivation, and improved measurement technology. Finally, the progress of quantum light sources applications in fundamental scientific problems and quantum network constructions are summarized, and prospects for practical applications and future development are discussed in brief.

Key words: deterministic solid-state quantum light source, molecular beam epitaxy, semiconductor quantum dot, single photon source, entangled photon source, quantum information technology

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